Scythia would be a good one too. More of a nomadic society from the northern portions of the Black and Caspian Seas, a city-state to represent them would be cool.
Since the Byzantine Empire is not yet a playable civilization (I'm crossing my fingers for a mod or DLC release) then Byzantium (the original Greek city) or Constantinople (which was basically just a city-state by the year it fell in 1453). Knossos, the Minoan city, would be cool.
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