Those will never go away. You get one per population point of the city. That is the main reason why happiness resources and civics matter. Hereditary Rule and Nationhood are good ways to raise the happy cap (the point where the > and you get angry citizens).
This is a feature that can't be solved. All cities have +X for overcrowding where X is the population. You just have to find sources of happiness. Check out Cabert's guide in the Strategy Articles forum on "Ways Into Happiness."
Secondly, check out Cabert's 'Ways into Happiness' article that delves into the happiness issue. "Overcrowding" is a natural negative relating to your city's size - you just need to find countering happiness approaches such as found through religion, culture, etc.
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