Not really, since those cities combined have less than a tenth of the US population. IIRC more than half of the population lives outside of major urban areas entirely. And why should major population centers be ignored and unpopulous states like New Mexico, Iowa and New Hampshire be the ones deciding the Presidency?
More importantly, people in Wyoming are represented 3.6 times more than people in California in the Electoral College. That doesn't sound like "One man, one vote" to me.
Wyoming: 170,000 people per Electoral vote (510,000 people/3 votes)
California: 615,820 people per Electoral vote (33,870,000 people/55 votes)
That is horribly unfair and horribly undemocratic.